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Laser plasma x-ray source for ultrafast time-resolved x-ray absorption spectroscopy

机译:用于超快时间分辨X射线吸收光谱的激光等离子体X射线源

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摘要

We describe a laser-driven x-ray plasma source designed for ultrafast x-ray absorption spectroscopy. The source is comprised of a 1 kHz, 20 W, femtosecond pulsed infrared laser and a water target. We present the x-ray spectra as a function of laser energy and pulse duration. Additionally, we investigate the plasma temperature and photon flux as we vary the laser energy. We obtain a 75 mu m FWHM x-ray spot size, containing similar to 10(6) photons/s, by focusing the produced x-rays with a polycapillary optic. Since the acquisition of x-ray absorption spectra requires the averaging of measurements from >10(7) laser pulses, we also present data on the source stability, including single pulse measurements of the x-ray yield and the x-ray spectral shape. In single pulse measurements, the x-ray flux has a measured standard deviation of 8%, where the laser pointing is the main cause of variability. Further, we show that the variability in x-ray spectral shape from single pulses is low, thus justifying the combining of x-rays obtained from different laser pulses into a single spectrum. Finally, we show a static x-ray absorption spectrum of a ferrioxalate solution as detected by a microcalorimeter array. Altogether, our results demonstrate that this water-jet based plasma source is a suitable candidate for laboratory-based time-resolved x-ray absorption spectroscopy experiments. (C) 2015 Author(s).
机译:我们描述了专为超快X射线吸收光谱设计的激光驱动X射线等离子体源。光源由1 kHz,20 W,飞秒脉冲红外激光和水靶组成。我们介绍了X射线光谱作为激光能量和脉冲持续时间的函数。此外,我们在改变激光能量时研究等离子体温度和光子通量。通过用多毛细管光学器件聚焦产生的X射线,我们获得了75微米的FWHM X射线光斑尺寸,包含类似于10(6)光子/ s的光斑。由于获取X射线吸收光谱需要对来自> 10(7)个激光脉冲的测量值求平均值,因此我们还提供了有关源稳定性的数据,包括X射线产量和X射线光谱形状的单脉冲测量。在单脉冲测量中,X射线通量的测量标准偏差为8%,其中激光指向是变化的主要原因。此外,我们表明,来自单个脉冲的x射线光谱形状的可变性较低,因此证明了将从不同激光脉冲获得的x射线组合为单个光谱是合理的。最后,我们显示了由微量量热仪阵列检测到的草酸亚铁溶液的静态X射线吸收光谱。总之,我们的结果表明,这种基于水射流的等离子体源是基于实验室的时间分辨X射线吸收光谱实验的合适候选者。 (C)2015年作者。

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